PUBLICATION

Design and biological assessment of membrane-tethering neuroprotective peptides derived from the pituitary adenylate cyclase-activating polypeptide type 1 receptor

Authors
de Molliens, M.P., Jamadagni, P., Létourneau, M., Devost, D., Hébert, T.E., Patten, S.A., Fournier, A., Chatenet, D.
ID
ZDB-PUB-190716-10
Date
2019
Source
Biochimica et biophysica acta. General subjects   1863(11): 129398 (Journal)
Registered Authors
Patten, Shumoogum
Keywords
BRET-based biosensor, Neuroprotection, PAC1 receptor, PACAP, Parkinson's disease, Pepducin
MeSH Terms
  • Animals
  • Cell Line, Tumor
  • Cell Survival/drug effects
  • HEK293 Cells
  • Humans
  • Neurogenesis/drug effects*
  • Neuroprotective Agents*/chemistry
  • Neuroprotective Agents*/pharmacology
  • Peptides*/chemistry
  • Peptides*/pharmacology
  • Receptors, Pituitary Adenylate Cyclase-Activating Polypeptide, Type I/chemistry*
  • Zebrafish/embryology*
PubMed
31306709 Full text @ BBA General Subjects
Abstract
The pituitary adenylate cyclase-activating polypeptide (PACAP) type 1 receptor (PAC1), a class B G protein-coupled receptor (GPCR), has emerged as a promising target for treating neurodegenerative conditions. Unfortunately, despite years of research, no PAC1-specific agonist has been discovered, as activity on two other GPCRs, VPAC1 and VPAC2, is retained with current analogs. Cell signaling is related to structural modifications in the intracellular loops (ICLs) of GPCRs. Thus, we hypothesized that peptides derived from the ICLs (called pepducins) of PAC1 might initiate, as allosteric ligands, signaling cascades after recognition of the parent receptor and modulation of its conformational landscape.
Three pepducins were synthesized and evaluated for their ability to 1) promote cell survival; 2) stimulate various signaling pathways associated with PAC1 activation; 3) modulate selectively PAC1, VPAC1 or VPAC2 activation; and 4) sustain mobility and prevent death of dopaminergic neurons in a zebrafish model of neurodegeneration.
Assays demonstrate that these molecules promoted SH-SY5Y cell survival, a human neuroblastoma cell line expressing PAC1, and activated signaling via Gαs and Gαq, with distinct potencies and efficacies. Also, PAC1-Pep1 and PAC1-Pep2 activated selectively PAC1-mediated Gαs stimulation. Finally, experiments, using a zebrafish neurodegeneration model, showed a neuroprotective action with all three pepducins and in particular, revealed the ability of PAC1-Pep1 and PAC1-Pep3 to preserve fish mobility and tyrosine hydroxylase expression in the brain.
We have developed the first neuroprotective pepducins derived from PAC1, a class B GPCR.
PAC1-derived pepducins represent attractive templates for the development of innovative neuroprotecting molecules.
Genes / Markers
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Human Disease / Model
Sequence Targeting Reagents
Fish
Antibodies
Orthology
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Mapping